A Macroscopic Probe of Quantum States

Physics 14, s95
A simple measurement of the magnetic susceptibility of a material can reveal the population of specific quantum states in the material.

The magnetic susceptibility of a material quantifies how much the material is magnetized when exposed to a magnetic field. This macroscopic property results from the contributions of many microscopic quantum states with nonzero magnetic moments. A typical susceptibility measurement, however, yields a value that averages over the statistical ensemble of all states—it cannot deliver information on the populations of specific quantum states. Now, a team at Cardiff University and University College London, both in the UK, shows that, in a particular magnetic system, a susceptibility measurement can directly probe the populations of two spin states [1]. The idea could allow researchers to use simple susceptibility measurements to study the quantum-state dynamics of exotic magnetic materials.

The researchers study a “dilute spin ice” consisting of ions arranged on a tetrahedral lattice. With a small number of these ions possessing a large electronic spin, the material can be described as a simple two-level (spin-up–spin-down) system. These spins, and their coupling to other excitations in the material, contribute to the measured susceptibility, and the different contributions can be isolated by changing the frequency of an applied magnetic field. In particular, above several kHz, the magnetic susceptibility is unaffected by slow relaxation mechanisms that involve spin-spin and spin-lattice interactions. With these mechanisms excluded, the team shows that the measured susceptibility is directly related to the difference between the populations of the spin-up and spin-down states. To create such a difference, they bring the system to temperatures as low as 76 mK. They then quantify the population imbalance from susceptibility measurements. The researchers suggest that next-generation susceptometers reaching MHz frequencies could make the technique applicable to more complex materials.

–Matteo Rini

Matteo Rini is the Editor of Physics.


  1. D. Billington et al., “Experimental measurement of the isolated magnetic susceptibility,” Phys. Rev. B 104, 014418 (2021).

Subject Areas

MagnetismMaterials ScienceStatistical PhysicsCondensed Matter PhysicsQuantum Physics

Related Articles

Magnons Dampen Skyrmion Motion

Magnons Dampen Skyrmion Motion

Adding a friction term to models helps them better account for how spin textures evolve experimentally at room temperature. Read More »

Quantum Metasurfaces Entangle Photons on Demand

Quantum Metasurfaces Entangle Photons on Demand

When it’s modulated by laser beams, a surface made of polarizable meta-atoms can entangle a photon’s properties in multiple, controllable ways. Read More »

Time Crystals in Open Systems
Quantum Physics

Time Crystals in Open Systems

Experiments successfully capture signatures of a discrete time crystal phase in an open, quantum many-body system. Read More »

More Articles