Synopsis: Never say never to a forbidden transition

A three-photon process provides a new route toward exciting surface plasmon polaritons on a flat metal surface.
Synopsis figure
Illustration: J. Renger et al., Phys. Rev. Lett. (2009)

Surface plasmon polaritons (SPPs) are electromagnetic waves that are coupled to charge density oscillations at a metal/dielectric interface, and result from light or free electrons hitting the metal surface. The study of SPPs is central to the burgeoning field of plasmonics. From optoelectronics to metamaterials, imaging, and biosensing, SPPs find important applications because they are highly localized at the surface and have well-defined resonant energies.

For a given frequency of light hitting a metal surface from air, the momentum associated with the SPP in the metal will always be greater than the in-plane momentum of the light, so how can one couple to the other? Up to now, the two standard ways of exciting an SPP on a metal with light have been to either use a nonpropagating, or “evanescent,” light wave, or to use a rough or artificially corrugated surface.

Writing in Physical Review Letters, a team of researchers from ICFO in Barcelona, Spain, and the Institute of Optics at the University of Rochester in the US theoretically propose and experimentally demonstrate a new route to SPP excitation from propagating light impinging directly on a flat surface of gold. Their method to produce this “free-space excitation” involves not one but three incident photons at a time, whose momenta add to give the right balance of in-plane momentum for SPP coupling.

These SPPs have well-defined energies, momenta, and directivity. The coupling efficiency is still much too weak for this technique to be practically viable, but the rationale behind this new method could be applied towards exciting other bound modes in related systems, such as surface phonon polaritons, waveguide modes, and excitations in 2D electron gases. – Manolis Antonoyiannakis


More Announcements »

Subject Areas


Previous Synopsis

Next Synopsis


The space between

Read More »

Related Articles

Synopsis: Hydrogen  Bonding Comes to the Rescue
Chemical Physics

Synopsis: Hydrogen Bonding Comes to the Rescue

Hydrogen bonding may safeguard biomolecules against the damaging effects of UV light. Read More »

Viewpoint: Cold Results from Fast Lasers

Viewpoint: Cold Results from Fast Lasers

Ultrafast lasers show promise to cool down and trap atomic species inaccessible to more traditional methods. Read More »

Viewpoint: Showtime for Molecular Movies

Viewpoint: Showtime for Molecular Movies

Molecular movies of vibrating iodine molecules have been recorded in time-resolved x-ray and electron diffraction experiments. Read More »

More Articles