Synopsis: A New Quantum Spin Liquid Candidate

Neutron scattering experiments reveal signatures of an exotic phase of matter in the pyrochlore magnet Ce2Zr2O7.
Synopsis figure
J. Gaudet et al., Phys Rev. Lett. (2019)

In the quest to realize the exotic phase of matter known as a quantum spin liquid—a state thought to harbor quasiparticles useful for reliable quantum computing—a promising new candidate material has emerged: the pyrochlore magnet Ce2Zr2O7. In this material, Jonathan Gaudet of McMaster University, Canada, and colleagues now find the hallmarks of the quantum spin liquid’s ground state, dubbed quantum spin ice. Their results suggest that Ce2Zr2O7 and other materials with similar chemical compositions might be excellent platforms for investigating the physics of this weird phase.

When most magnetic materials are cooled to low temperatures, the spins of their electrons align in some manner. However, in quantum spin liquids, the spins remain disordered, even at absolute zero. Gaudet and colleagues identified Ce2Zr2O7 as a promising spin liquid candidate because it possesses well-characterized magnetic moments that are known to stay disordered down to about 50 mK.

Gaudet and colleagues synthesized samples of Ce2Zr2O7 and used neutron scattering experiments to reveal the spins’ arrangement in the material. The team reports that at a temperature of 60 mK, the neutron scattering patterns closely match those predicted for a quantum spin ice (see 30 August 2012 Synopsis).

A quantum spin ice can host a variety of exotic quasiparticles, such as electric and magnetic monopoles and “emergent photons”—photon-like excitations that arise from complex interactions between many electrons. The team hopes that Ce2Zr2O7 will become a reliable system for stabilizing these quasiparticles, allowing researchers to easily study their properties in a self-contained quantum electrodynamic system.

This research is published in Physical Review Letters.

–Christopher Crockett

Christopher Crockett is a freelance writer based in Arlington, Virginia.


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